Hi mdauphin,
It looks like you would like to perform low/register level programming with the VME-MXI-2. One way you can do this is through the VISA Interactive Control. You can do this by using the Register I/O pane. There is more information about this here
LabVIEW also ships with some example code that you may use. You can open the example finder by going to Help > Find Examples. Once there, browse to Hardware Input and Output > VISA > Low Level Register Access. There is also a High Level Register Access example.
Rasheel