I wouldn't use anything BUT LabVIEW for this, and I have.
I created an automated test setup to take several hundred measurements including all of the RF measurements, voltages, resistance, even Audio levels, and a host of others using ONLY a Laptop with LabVIEW, and several instruments communicating through a GPIB-USB converter.
Of course, if I had to do it over again, I would have used PXI.