Your initial parameters are far from appropriate values. When I plot the formula you want to fit with the x data the graph does not remotely resemble the data graph. Altenbach asked about this in your other thread.
Note the orders of magnitude difference in the Y-axes.
I looked at the formula and saw that to get a peak the value of a1 had to be between 300 and 400. Then I ddjsuted the other parameters until the curve began to resemble the data.
Again, as altenbach suggested, I switched to using a VI to calculate the model function. When I ran it that way, I got an error stating that the maximum number of iterations had been exceeded. On your VI you had set the termination parameters to 1 iteration maximum and tolerance of 1E-14. Considering that Lev-Mar is an iterative process and that your data has ~2% noise and the peak is not really symmetric, those values guarantee that it will never find a solution. I changed maximum iterations to 100 and tolerance to 1E-4. It converged and produced the result shown below.
The model function VI looks like this. See the Detailed help for Lev-Mar for information about creating this VI.
Lynn